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JNC TJ9400 2000-004, 109 Pages, 2000/02
We estimated covariances of the JENDL-3.2 data on the nuclides and reactions needed to analyze fast-reactor cores for the past three years, and produced covariance files. The present work was undertaken to re-examine the covariance files and to make some improvements. The covariances improved are the ones for the inelastic scattering cross section of O, the total cross section of Na, the fission cross section of U, the capture cross section of U, and the resolved resonance parameters for U. Moreover, the covariances of U data were newly estimated by the present work. The covariances obtained were compiled in the ENDF-6 format.
Sato, Haruo; ; ; *; *; Yui, Mikazu
PNC TN8410 97-127, 57 Pages, 1997/08
Retardation of key nuclides is one of the most important mechanisms to be examined specifically and modelled for the performance assessment of geological disposal of radioactive waste. We have been studing diffusion of nuclides into the pore spaces of the rock matrix, sorption of nuclides on the rock pore surfaces and pore properties to quantify the degree of nuclide retardation in fractured crystalline rock. The work has concentrated on predominant water conducting fracture system in the host granodiorite in the Kamaishi In Situ Test Site, which consists of fracture fillings and altered granodiorite. Through-diffusion experiements to obtain effective and apparent diffusion coefficients (Da and De, respectively) for Na, Cs, HTO, Cl and Se as a function of ionic charge at 22 25C and batch sorption experiments for Cs, Sr, Se, U and Pu were conducted on fracture fillings, altered and intact granodiorite. The experiments only for Se, a redox sensitive element, were done in an N2-atmospheric glove box (O 1 ppm) to keep the chemical species. In situ groundwater (pH8.79.5) sampled from the same place as rock samples was used for the experiments. Porosity and density of cach rock sample were determined by both water saturation method and mercury porosimetry, and pore-size distribution and specific surface area of pores were measured by mercury porosimetry. The porosity is in the order; fracture fillings (5.6%) altered rock (3.2%) intact rock (2.3%). The pore-size distribution of the intact and altered granodiorite is ranging from 10 nm to 0.2 mm, and the fracture fillings have that of 50 nm to 0.2 mm, but a lot of pores were found around 100 nm and 0.2 mm in the fracture fillings. The effective diffusion coefficients for all species (Na, Cs, HTO, Cl, Se0) are in the order of fracture fillings altered rock intact rock in proportion to these porosities. Effective diffusion ...
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PNC TN9450 96-052, 694 Pages, 1996/10
The present report compiles the experimental data of JUPITER Phase-II, which was a joint research program between U.S. DOE and PNC of Japan, using the ZPPR facility, which stands for Zero Power Physics Reactor at ANL-Idaho in l982 to l984. The JUPITER-II experiment was a series of critical experiments for conventional radial heterogeneous cores of 650 MWe class LMFBR, including six experimental cores. The nuclear characteristics recorded here include criticality, control rod reactivity, reaction rate distribution, sodium void reactivity, sample reactivity, Doppler reactivity and gamma heating. The present work is a part of efforts to develop a standard data base for LMFBR core nuclear design at PNC. The detail of experimental data is thoroughly recorded here so as to re-analyze these experiments in future. In addition, these experimental data are installed in the computer system at OEC for convenience of analytical code input.